Published in

American Association for the Advancement of Science, Science Advances, 18(6), p. eaay9709, 2020

DOI: 10.1126/sciadv.aay9709

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Three-dimensional magnetism and the Dzyaloshinskii-Moriya interaction in S = 3/2 kagome staircase Co3V2O8

This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

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Abstract

Time-of-flight neutron data reveal spin waves in the ferromagnetic ground state of the kagome staircase material Co3V2O8. While previous work has treated this material as quasi–two-dimensional, we find that an inherently three-dimensional description is needed to describe the spin wave spectrum throughout reciprocal space. Moreover, spin wave branches show gaps that point to an unexpectedly large Dzyaloshinskii-Moriya interaction on the nearest-neighbor bond, with D1 ≥ J1/2. A better understanding of the Dzyaloshinskii-Moriya interaction in this material should shed light on the multiferroicity of the related Ni3V2O8. At a higher temperature where Co3V2O8 displays an antiferromagnetic spin density wave structure, there are no well-defined spin wave excitations, with most of the spectral weight observed in broad diffuse scattering centered at the (0, 0.5, 0) antiferromagnetic Bragg peak.

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